Correlation between deep-level defects and functional properties of β-(SnxGa1-x)2O3 on Si photodetectors

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Hatipoglu, Isa and Hunter, Daniel A. and Mukhopadhyay, Partha and Williams, Martin S. and Edwards, Paul R. and Martin, Robert W. and Schoenfeld, Winston V. and Gunasekar, G. Naresh (2021) Correlation between deep-level defects and functional properties of β-(SnxGa1-x)2O3 on Si photodetectors. Journal of Applied Physics, 130 (20). 204501. ISSN 0021-8979 (https://doi.org/10.1063/5.0068186)

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Abstract

Heterogeneous integration of β-(Sn xGa1− x)2O3 (TGO) UV-C photodetectors on silicon substrates by molecular beam epitaxy is demonstrated. Multimodal electron microscopy and spectroscopy techniques reveal a direct correlation between structural, compositional, and optical properties of TGO and the functional properties of the photodetectors. Wavelength dispersive x-ray spectroscopy results accurately determine Sn concentrations ( x) in the region of 0.020, and room temperature cathodoluminescence (CL) hyperspectral imaging shows changes in the CL emission intensity in TGO compared with a Ga2O3 sample with no Sn. Alloying Ga2O3 with Sn is shown to quench the red emission and enhance the blue emission. The increase in blue emission corresponds to the rise in VGa-related deep acceptors responsible for the high gain observed in the TGO detectors. A Ga2O3 nucleation layer is shown to improve the TGO surface quality and give better device properties compared to TGO grown directly onto the Si substrate, including a higher specific detectivity on the order of 1012 Jones.

ORCID iDs

Hatipoglu, Isa, Hunter, Daniel A., Mukhopadhyay, Partha, Williams, Martin S., Edwards, Paul R. ORCID logoORCID: https://orcid.org/0000-0001-7671-7698, Martin, Robert W. ORCID logoORCID: https://orcid.org/0000-0002-6119-764X, Schoenfeld, Winston V. and Gunasekar, G. Naresh ORCID logoORCID: https://orcid.org/0000-0002-9642-8137;
  • Item type:Article
    ID code:78496
    Dates:
    Date
    Event
    28 November 2021
    Published
    4 November 2021
    Accepted
    23 August 2021
    Submitted
    Subjects:Science > Physics
    Department:Faculty of Science > Physics
    Depositing user: Pure Administrator
    Date deposited:10 Nov 2021 15:42
    Last modified:05 Dec 2024 08:24
    URI:https://strathprints.strath.ac.uk/id/eprint/78496
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