Ultrafast dynamics in complex fluids observed through the ultrafast optically-heterodyne-detected optical-Kerr-effect (OHD-OKE)

Hunt, Neil T. and Jaye, Andrew A. and Meech, Stephen R. (2007) Ultrafast dynamics in complex fluids observed through the ultrafast optically-heterodyne-detected optical-Kerr-effect (OHD-OKE). Physical Chemistry Chemical Physics, 9 (18). pp. 2167-2180. ISSN 1463-9076 (https://doi.org/10.1039/b616078f)

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Abstract

The ultrafast molecular dynamics of complex fluids have been recorded using the optically-heterodyne-detected optical-Kerr-effect (OHD-OKE). The OHD-OKE method is reviewed and some recent refinements to the method are described. Applications to a range of complex fluids, including microemulsions, polymer melts and solutions, liquid crystal and ionic liquids are surveyed. The level of detail attainable with the OHD-OKE method in these complex fluids is discussed. The prospects for future experiments are discussed.