Quantifying the strength and asymmetry of giant resonances in the photorecombination of Sc3+ and the photoionization of Sc2+

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Nikolic, D. and Gorczyca, T.W. and Badnell, N.R. (2010) Quantifying the strength and asymmetry of giant resonances in the photorecombination of Sc3+ and the photoionization of Sc2+. Physical Review A, 81. 030501. ISSN 1050-2947 (http://dx.doi.org/10.1103/PhysRevA.81.030501)

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Abstract

We report on strong interference effects for the dominant, highly correlated, broad, and asymmetric 3p53d2(2F5/2,7/2o) giant resonances in the photorecombination of Sc3+. Using a nonorthogonal perturbative multiconfiguration Breit-Pauli approach, we present theoretical photorecombination cross sections that are in line with the Test Storage Ring measurements of Schippers et al. In order to reproduce the observed asymmetric resonance profiles near threshold, it was necessary to include resonance-continuum interference. Also, we present Sc2+ photoionization cross sections that agree with the Advance Light Source measurements of Schippers et al. This perturbative method is based on analytical expressions for the cross sections in terms of computed energies and transition rates, thereby directly determining resonance strengths and Fano asymmetry parameters. Of particular note, our reported absolute cross sections are in excellent agreement with experimental results, in contrast to all previous theoretical calculations. Furthermore, the apparent violation of the sum rule prediction, determined both from our integrated photoionization cross sections and from experimental results, is found to be due to radiative damping of narrow resonances.

ORCID iDs

Nikolic, D., Gorczyca, T.W. and Badnell, N.R. ORCID logoORCID: https://orcid.org/0000-0001-7418-7996;
  • Item type:Article
    ID code:26866
    Dates:
    Date
    Event
    5 March 2010
    Published
    Subjects:Science > Physics
    Department:Faculty of Science > Physics
    Depositing user:Users 1261 not found.
    Date deposited:19 Aug 2010 12:15
    Last modified:11 Nov 2024 09:36
    Related URLs:
    URI:https://strathprints.strath.ac.uk/id/eprint/26866
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