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Open Access research with a European policy impact...

The Strathprints institutional repository is a digital archive of University of Strathclyde's Open Access research outputs. Strathprints provides access to thousands of Open Access research papers by Strathclyde researchers, including by researchers from the European Policies Research Centre (EPRC).

EPRC is a leading institute in Europe for comparative research on public policy, with a particular focus on regional development policies. Spanning 30 European countries, EPRC research programmes have a strong emphasis on applied research and knowledge exchange, including the provision of policy advice to EU institutions and national and sub-national government authorities throughout Europe.

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Modelling and simulation of the flux responses of a gas-solid catalytic micro-reactor

Buffham, B.A. and Hellgardt, K. and Heslop, M. and Mason, G. and Richardson, D.J. (2002) Modelling and simulation of the flux responses of a gas-solid catalytic micro-reactor. Chemical Engineering Science, 57 (6). pp. 953-966. ISSN 0009-2509

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Abstract

The usual explanation of how a solid catalyst promotes a gas-phase reaction is that adsorption is followed by reaction and desorption. This composite process may be followed by measuring the flow-rate changes (the flux response) caused by adsorption, reaction and desorption in a continuous-flow reactor. The mathematical modelling of the flux responses of gas-solid catalytic reactors is discussed. A numerical simulator has been developed that allows flux responses to be calculated. Examples are given and the simulator is tested against an analytical special case. The salient points of simulated flux responses are similar to those of preliminary experimental flux responses. The combination of the mathematical model with a specially designed series of experiments could allow reaction, adsorption and mass-transfer rate coefficients to be determined.