Organic polariton lasing and the weak to strong coupling crossover
Strashko, Artem and Kirton, Peter and Keeling, Jonathan (2018) Organic polariton lasing and the weak to strong coupling crossover. Physical Review Letters, 121 (19). 193601. ISSN 1079-7114 (https://doi.org/10.1103/PhysRevLett.121.193601)
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Abstract
Following experimental realizations of room temperature polariton lasing with organic molecules, we present a microscopic model that allows us to explore the crossover from weak to strong matter-light coupling. We consider a nonequilibrium Dicke-Holstein model, including both strong coupling to vibrational modes and strong matter-light coupling, providing the phase diagram of this model in the thermodynamic limit. We discuss the mechanism of polariton lasing, uncovering a process of self-tuning, and identify the relation and distinction between regular dye lasers and organic polariton lasers.
ORCID iDs
Strashko, Artem, Kirton, Peter ORCID: https://orcid.org/0000-0002-3915-1098 and Keeling, Jonathan;-
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Item type: Article ID code: 71354 Dates: DateEvent9 November 2018Published24 October 2018AcceptedNotes: © 2018, American Physical Society. This work has been made available online in accordance with the publisher’s policies. This is the author created accepted version manuscript following peer review and as such may differ slightly from the final published version. The final published version of this work is available at https://doi.org/10.1103/PhysRevLett.121.193601 Subjects: Science > Physics Department: UNSPECIFIED Depositing user: Pure Administrator Date deposited: 05 Feb 2020 14:18 Last modified: 11 Nov 2024 12:35 Related URLs: URI: https://strathprints.strath.ac.uk/id/eprint/71354