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Strathprints serves world leading Open Access research by the University of Strathclyde, including research by the Strathclyde Institute of Pharmacy and Biomedical Sciences (SIPBS), where research centres such as the Industrial Biotechnology Innovation Centre (IBioIC), the Cancer Research UK Formulation Unit, SeaBioTech and the Centre for Biophotonics are based.

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New evidence for the influence of step morphology on the formation of Au atomic chains on vicinal Si(111) surfaces

McAlinden, N. and McGilp, J. F. (2010) New evidence for the influence of step morphology on the formation of Au atomic chains on vicinal Si(111) surfaces. EPL: A Letters Journal Exploring the Frontiers of Physics, 92 (6). -. ISSN 0295-5075

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Abstract

Gold atomic chain structures that grow on singular and vicinal Si(111) surfaces have attracted considerable interest as model systems for exploring quasi-one-dimensional metallic behaviour. The structure of the prototypical Si(111)-5 x 2-Au system remains controversial, however. Reflection anisotropy spectroscopy provides new, independent evidence supporting a recently proposed three-Au-chain structure. For stepped surfaces, the results provide good evidence that a single Au chain forms adjacent to [(1) over bar(1) over bar2] steps and a double Au chain forms adjacent to [11 (2) over bar] steps. In both cases spectral lineshape and coverage data support a three-chain Si(111)-5 x 2-Au structure forming over the remainder of the terrace. For all the vicinal Si(111) surfaces, including Si(557) and Si(775), it is the step morphology, and not the terrace width, that determines whether single- or double-Au-chain structures are formed in the region of the steps.